Supplementary material Table 1. The Dunham coefficients that describe the A$^1\Sigma^+$ state of $^{39}$K$^7$Li in the range $0 \leq v' \leq 34$, $9 \leq J' \leq 73$. The numbers in parentheses correspond to one standard deviation in units of the last digits. Values of the coefficients are in \rcm, except for $R_e$ in \AA. experiment theory [21] Y ( 0, 0) 12097.11(3) 12056 Y ( 1, 0) 137.0821(131) 135.5 Y ( 2, 0) -0.98904(221) Y ( 3, 0) 0.2559(16)D-01 Y ( 4, 0) -0.511(5)D-03 Y ( 5, 0) 0.388(6)D-05 Y ( 0, 1) 0.182043(29) 0.1837 Y ( 1, 1) -0.20751(46)D-02 Y ( 2, 1) 0.4189(31)D-04 Y ( 3, 1) -0.575(7)D-06 Y ( 0, 2) -0.1264(6)D-05 Y ( 1, 2) 0.164(4)D-07 De 7105.0(1) 7186 Re 3.9466(3) 3.916 Table 2. Rotationless RKR potential energy curve for the A$^1\Sigma^+$ state of KLi. The equilibrium distance, $R_e$, equals to 3.9466~\AA. v Gv Rmin Rmax 0 68.319 3.7553 4.1633 1 203.503 3.6292 4.3400 2 336.926 3.5485 4.4710 3 468.716 3.4862 4.5832 4 598.993 3.4345 4.6844 5 727.865 3.3900 4.7781 6 855.430 3.3506 4.8661 7 981.776 3.3152 4.9498 8 1106.983 3.2829 5.0299 9 1231.121 3.2533 5.1070 10 1354.251 3.2258 5.1815 11 1476.429 3.2001 5.2538 12 1597.702 3.1760 5.3242 13 1718.108 3.1533 5.3928 14 1837.681 3.1318 5.4598 15 1956.450 3.1114 5.5255 16 2074.436 3.0919 5.5899 17 2191.656 3.0734 5.6533 18 2308.122 3.0556 5.7156 19 2423.843 3.0385 5.7771 20 2538.824 3.0221 5.8378 21 2653.065 3.0063 5.8978 22 2766.566 2.9911 5.9572 23 2879.322 2.9764 6.0161 24 2991.330 2.9622 6.0745 25 3102.581 2.9485 6.1326 26 3213.069 2.9353 6.1904 27 3322.786 2.9225 6.2479 28 3431.723 2.9102 6.3053 29 3539.874 2.8983 6.3626 30 3647.232 2.8868 6.4198 31 3753.793 2.8757 6.4769 32 3859.554 2.8651 6.5341 33 3964.514 2.8549 6.5914 34 4068.675 2.8452 6.6487 Table 3. Transitions in the B1Pi <-- X1Sigma+ band system of 39K7Li excited by the probe (labelling) laser Laser wave number Labelled transition 17498.47 cm-1 (0,31) <- (0,30) 17464.35 cm-1 (0,41) <- (0,40) (0,36) <- (0,36) 17474.27 cm-1 (0,29) <- (0,30) 17504.19 cm-1 (0,19) <- (0,20) (0,29) <- (0,28) (2,61) <- (0,62) 17515.63 cm-1 (0,14) <- (0,15) (1,46) <- (0,47) (3,73) <- (0,72) 17418.67 cm-1 (0,51) <- (0,50) 17371.82 cm-1 (1,34) <- (1,35) 17429.96 cm-1 (1,26) <- (1,25) (1,66) <- (0,65) (1,17) <- (1,18) 17356.41 cm-1 (1,46) <- (1,45) 17445.91 cm-1 (0,36) <- (0,37) (1,64) <- (0,63) (1,18) <- (1,17) (1,9) <- (1,10) 17105.96 cm-1 (0,21) <- (2,20) (2,15) <- (2,15) (2,28) <- (3,29) (2,32) <- (3,32) 17096.27 cm-1 (0,26) <- (2,25) (2,16) <- (2,17) (1,48) <- (2,49) 17082.94 cm-1 (0,32) <- (2,31) 17071.23 cm-1 (0,36) <- (2,35) (1,52) <- (2,53) (2,36) <- (3,37) 17050.61 cm-1 (0,42) <- (2,41) (0,32) <- (2,33) 17093.95 cm-1 (2,17) <- (2,18) (2,27) <- (2,26) (2,28) <- (2,27) (2,31) <- (3,32) (2,35) <- (3,35) (0,66) <- (1,66) 17061.40 cm-1 (2,29) <- (2,30) (2,39) <- (2,38) (2,38) <- (3,39) 17419.15 cm-1 (1,21) <- (1,22) (1,30) <- (1,29) (2,46) <- (1,47) 17395.63 cm-1 (1,37) <- (1,36) (1,28) <- (1,29) 17370.65 cm-1 (1,43) <- (1,42) (2,60) <- (1,59) 17081.71 cm-1 (2,22) <- (2,23) (2,42) <- (3,41) Table 4. Observed line positions (in cm-1) in the A1Sigma+ <-- X1Sigma+ band system of 39K7Li vs. positions calculated from the Dunham coefficients of the A nad X states. Lines used in the fit of Dunham coefficients. v' J' v" J" obs. calc. obs.-calc. 4 16 0 15 12576.05000 12576.03142 .018578 5 14 0 15 12693.95000 12693.82563 .124373 5 16 0 15 12704.60000 12704.44218 .157818 10 14 0 15 13318.63000 13318.62078 .009222 10 16 0 15 13328.73000 13328.76891 -.038906 5 19 0 20 12677.14000 12676.93796 .202045 5 21 0 20 12691.18000 12690.94456 .235437 6 19 0 20 12803.63000 12803.88395 -.253954 6 21 0 20 12817.57000 12817.75764 -.187640 7 19 0 20 12929.70000 12929.63468 .065322 7 21 0 20 12943.42000 12943.38047 .039525 9 19 0 20 13177.71000 13177.85289 -.142893 9 21 0 20 13191.28000 13191.35688 -.076879 10 19 0 20 13300.50000 13300.45022 .049784 10 21 0 20 13313.87000 13313.83971 .030286 6 27 0 28 12767.43000 12767.58515 -.155149 6 29 0 28 12786.68000 12786.76954 -.089539 7 27 0 28 12892.82000 12892.75127 .068731 7 29 0 28 12911.80000 12911.75933 .040671 9 27 0 28 13139.81000 13139.86432 -.054322 9 29 0 28 13158.52000 13158.53914 -.019141 10 27 0 28 13262.01000 13261.93849 .071509 10 29 0 28 13280.50000 13280.45561 .044388 6 29 0 30 12756.78000 12756.82223 -.042231 6 31 0 30 12777.25000 12777.31958 -.069580 7 29 0 30 12881.90000 12881.81202 .087978 7 31 0 30 12902.22000 12902.12114 .098861 9 29 0 30 13128.61000 13128.59183 .018167 9 31 0 30 13148.60000 13148.54527 .054731 9 29 0 30 13128.61000 13128.59183 .018167 9 31 0 30 13148.51000 13148.54527 -.035269 10 29 0 30 13250.56000 13250.50830 .051696 10 31 0 30 13270.39000 13270.29345 .096553 10 29 0 30 13250.58000 13250.50830 .071696 10 31 0 30 13270.39000 13270.29345 .096553 5 35 0 36 12595.16000 12594.98362 .176376 5 37 0 36 12619.59000 12619.60971 -.019707 6 35 0 36 12720.53000 12720.51467 .015331 6 37 0 36 12744.94000 12744.90846 .031542 7 35 0 36 12845.08000 12844.90445 .175547 7 37 0 36 12869.25000 12869.07491 .175092 9 37 0 36 13114.35000 13114.29934 .050662 10 35 0 36 13212.10000 13211.93088 .169117 10 37 0 36 13235.61000 13235.48007 .129932 11 35 0 36 13332.26000 13332.41827 -.158271 11 37 0 36 13355.76000 13355.77493 -.014930 2 36 0 37 12204.54000 12204.50671 .033293 2 38 0 37 12230.63000 12230.55673 .073275 3 36 0 37 12333.92000 12333.87568 .044317 3 38 0 37 12359.69000 12359.65668 .033320 4 36 0 37 12461.89000 12461.82686 .063144 4 38 0 37 12487.47000 12487.34959 .120407 5 36 0 37 12588.33000 12588.46389 -.133894 5 38 0 37 12613.63000 12613.73861 -.108613 5 36 0 37 12588.39000 12588.46389 -.073894 5 38 0 37 12613.70000 12613.73861 -.038613 6 36 0 37 12713.78000 12713.88030 -.100296 6 38 0 37 12738.89000 12738.91672 -.026720 7 36 0 37 12838.16000 12838.15986 .000145 7 38 0 37 12863.18000 12862.96719 .212808 8 36 0 37 12961.16000 12961.37713 -.217128 9 36 0 37 13083.56000 13083.59790 -.037898 9 38 0 37 13107.95000 13107.97261 -.022610 10 38 0 37 13229.25000 13229.04978 .200218 10 38 0 37 13229.26000 13229.04978 .210218 11 36 0 37 13325.12000 13325.27200 -.151999 11 38 0 37 13349.14000 13349.24470 -.104701 11 36 0 37 13325.10000 13325.27200 -.171999 11 38 0 37 13349.13000 13349.24470 -.114701 12 36 0 37 13444.81000 13444.81723 -.007227 12 38 0 37 13468.56000 13468.59911 -.039111 13 36 0 37 13563.69000 13563.55068 .139322 13 38 0 37 13587.23000 13587.14785 .082154 14 36 0 37 13681.50000 13681.50126 -.001262 14 38 0 37 13704.92000 13704.91930 .000704 15 36 0 37 13798.73000 13798.69191 .038092 15 38 0 37 13822.02000 13821.93587 .084125 16 36 0 37 13915.22000 13915.14003 .079967 17 36 0 37 14030.94000 14030.85801 .081989 17 38 0 37 14053.83000 14053.76697 .063029 6 39 0 40 12693.03000 12692.98351 .046487 6 41 0 40 12720.01000 12719.93512 .074877 7 41 0 40 12843.74000 12843.62059 .119408 8 39 0 40 12939.68000 12939.79771 -.117710 10 41 0 40 13208.74000 13208.68828 .051725 11 39 0 40 13302.71000 13302.75982 -.049818 6 46 0 47 12638.40000 12638.46863 -.068634 6 48 0 47 12669.73000 12669.80769 -.077694 7 46 0 47 12761.34000 12761.48984 -.149841 7 48 0 47 12792.43000 12792.54403 -.114026 8 46 0 47 12883.37000 12883.49684 -.126842 8 48 0 47 12914.13000 12914.27716 -.147159 10 46 0 47 13124.47000 13124.71160 -.241598 10 48 0 47 13154.75000 13154.97457 -.224573 11 46 0 47 13243.92000 13244.02074 -.100737 11 48 0 47 13273.92000 13274.03893 -.118929 12 46 0 47 13362.57000 13362.51937 .050628 6 49 0 50 12612.59000 12612.65980 -.069797 6 51 0 50 12645.76000 12645.84073 -.080730 7 49 0 50 12735.18000 12735.24966 -.069657 7 51 0 50 12768.05000 12768.12967 -.079673 8 49 0 50 12856.77000 12856.84199 -.071994 8 51 0 50 12889.42000 12889.43279 -.012795 10 49 0 50 13097.11000 13097.27350 -.163496 10 51 0 50 13129.19000 13129.31818 -.128181 11 49 0 50 13216.12000 13216.21206 -.092058 11 51 0 50 13247.89000 13247.99845 -.108450 12 49 0 50 13334.24000 13334.35282 -.112824 7 63 0 62 12655.34000 12655.53033 -.190334 8 61 0 62 12735.21000 12735.32057 -.110569 8 63 0 62 12774.83000 12774.89346 -.063465 9 61 0 62 12854.16000 12854.16748 -.007476 9 63 0 62 12893.45000 12893.40718 .042819 11 61 0 62 13089.43000 13089.46044 -.030440 11 63 0 62 13128.09000 13128.07117 .018829 12 61 0 62 13205.96000 13205.98149 -.021485 12 63 0 62 13244.38000 13244.29471 .085292 13 61 0 62 13321.82000 13321.79041 .029594 13 63 0 62 13359.87000 13359.81629 .053712 1 62 0 63 11865.53000 11865.55911 -.029114 1 64 0 63 11908.49000 11908.49204 -.002035 2 62 0 63 11991.63000 11991.75272 -.122717 2 64 0 63 12034.20000 12034.23290 -.032901 3 62 0 63 12116.58000 12116.60773 -.027733 3 64 0 63 12158.65000 12158.65427 -.004275 4 64 0 63 12282.07000 12281.86070 .209299 5 64 0 63 12403.84000 12403.94609 -.106089 6 62 0 63 12484.18000 12484.14275 .037252 6 64 0 63 12525.18000 12524.99418 .185822 7 64 0 63 12645.23000 12645.07900 .150997 7 64 0 65 12582.20000 12582.08191 .118091 8 64 0 65 12701.21000 12701.26827 -.058268 8 66 0 65 12742.49000 12742.51444 -.024443 9 66 0 65 12860.60000 12860.51248 .087520 10 64 0 65 12937.19000 12937.16138 .028620 11 66 0 65 13094.28000 13094.20346 .076535 12 64 0 65 13169.97000 13170.02774 -.057735 12 66 0 65 13210.11000 13209.96698 .143015 13 64 0 65 13285.49000 13285.40299 .087009 13 66 0 65 13325.10000 13325.04441 .055588 8 71 0 72 12616.41000 12616.20389 .206107 8 73 0 72 12661.03000 12661.22815 -.198152 9 71 0 72 12733.08000 12733.30181 -.221808 9 73 0 72 12778.08000 12777.95242 .127581 14 73 0 72 13351.42000 13351.20753 .212467 11 9 1 10 13244.97000 13244.99165 -.021652 12 9 1 10 13366.14000 13366.14523 -.005233 12 11 1 10 13372.89000 13372.91940 -.029404 13 9 1 10 13486.36000 13486.43652 -.076520 13 11 1 10 13493.06000 13493.15718 -.097184 14 9 1 10 13605.86000 13605.89871 -.038708 14 11 1 10 13612.50000 13612.56743 -.067427 15 9 1 10 13724.63000 13724.55901 .070987 15 11 1 10 13731.20000 13731.17721 .022795 16 9 1 10 13842.24000 13842.43914 -.199138 17 9 1 10 13959.48000 13959.55574 -.075741 17 11 1 10 13966.01000 13966.07656 -.066557 18 9 1 10 14076.03000 14075.92090 .109102 18 11 1 10 14082.51000 14082.39457 .115425 0 16 1 17 11821.46000 11821.61906 -.159056 0 18 1 17 11834.11000 11834.23621 -.126209 1 16 1 17 11956.18000 11956.26282 -.082822 1 18 1 17 11968.67000 11968.74114 -.071137 2 16 1 17 12089.29000 12089.16573 .124271 2 18 1 17 12101.62000 12101.51071 .109290 3 18 1 17 12232.47000 12232.67375 -.203747 4 16 1 17 12350.27000 12350.25411 .015891 4 18 1 17 12362.34000 12362.34797 -.007969 5 16 1 17 12478.89000 12478.66487 .225132 5 18 1 17 12490.87000 12490.64046 .229542 6 18 1 17 12617.40000 12617.64813 -.248130 10 16 1 17 13102.99000 13102.99159 -.001592 10 18 1 17 13114.41000 13114.43907 -.029071 10 18 1 17 13114.46000 13114.43907 .020929 11 16 1 17 13224.70000 13224.80022 -.100221 11 18 1 17 13236.12000 13236.15303 -.033035 11 16 1 17 13224.80000 13224.80022 -.000221 11 18 1 17 13236.18000 13236.15303 .026965 12 16 1 17 13345.67000 13345.71495 -.044950 12 18 1 17 13356.90000 13356.97619 -.076187 12 16 1 17 13345.66000 13345.71495 -.054950 12 18 1 17 13356.93000 13356.97619 -.046187 13 16 1 17 13465.75000 13465.77479 -.024789 13 18 1 17 13476.89000 13476.94730 -.057297 14 16 1 17 13584.95000 13585.01230 -.062302 14 18 1 17 13596.05000 13596.09869 -.048686 15 16 1 17 13703.43000 13703.45408 -.024079 15 18 1 17 13714.53000 13714.45670 .073296 16 16 1 17 13821.04000 13821.12119 -.081195 17 16 1 17 13938.07000 13938.02968 .040321 17 18 1 17 13948.84000 13948.87091 -.030911 18 16 1 17 14054.39000 14054.19098 .199019 18 18 1 17 14064.94000 14064.95410 -.014096 10 17 1 18 13099.39000 13099.42668 -.036683 10 19 1 18 13111.50000 13111.52249 -.022489 11 17 1 18 13221.13000 13221.18931 -.059312 11 19 1 18 13233.07000 13233.18513 -.115130 12 17 1 18 13342.01000 13342.05954 -.049541 12 19 1 18 13353.81000 13353.95864 -.148637 10 21 1 22 13083.41000 13083.38604 .023962 10 23 1 22 13098.09000 13098.06493 .025067 11 21 1 22 13204.94000 13204.93809 .001907 11 23 1 22 13219.53000 13219.49587 .034133 12 21 1 22 13325.64000 13325.60463 .035368 12 23 1 22 13340.06000 13340.04526 .014745 13 21 1 22 13445.40000 13445.42401 -.024008 13 23 1 22 13459.70000 13459.75114 -.051142 14 21 1 22 13564.39000 13564.42813 -.038131 14 23 1 22 13578.64000 13578.64513 -.005126 6 24 1 25 12574.08000 12574.22303 -.143025 6 26 1 25 12591.30000 12591.42625 -.126246 8 24 1 25 12824.20000 12823.93455 .265454 8 26 1 25 12841.10000 12840.82705 .272947 9 24 1 25 12947.14000 12947.20158 -.061582 10 26 1 25 13086.08000 13086.09626 -.016260 11 24 1 25 13190.87000 13190.85869 .011315 11 26 1 25 13207.27000 13207.32592 -.055916 11 24 1 25 13190.94000 13190.85869 .081315 11 26 1 25 13207.31000 13207.32592 -.015916 12 24 1 25 13311.26000 13311.34570 -.085702 12 26 1 25 13327.62000 13327.68065 -.060645 12 24 1 25 13311.35000 13311.34570 .004298 12 26 1 25 13327.65000 13327.68065 -.030645 13 24 1 25 13431.02000 13430.99117 .028830 13 26 1 25 13447.22000 13447.19797 .022026 14 24 1 25 13549.84000 13549.82652 .013478 14 26 1 25 13565.92000 13565.90898 .011016 11 28 1 29 13169.78000 13169.57905 .200948 11 30 1 29 13188.44000 13188.57356 -.133563 11 28 1 29 13169.74000 13169.57905 .160948 11 30 1 29 13188.43000 13188.57356 -.143563 12 28 1 29 13289.80000 13289.79150 .008499 12 30 1 29 13308.64000 13308.63383 .006175 12 28 1 29 13289.78000 13289.79150 -.011501 12 30 1 29 13308.61000 13308.63383 -.023825 13 28 1 29 13409.18000 13409.17102 .008977 13 30 1 29 13427.91000 13427.86596 .044040 13 28 1 29 13409.14000 13409.17102 -.031023 13 30 1 29 13427.87000 13427.86596 .004040 14 28 1 29 13527.75000 13527.74832 .001679 14 28 1 29 13527.74000 13527.74832 -.008321 9 34 1 35 12890.23000 12890.27222 -.042219 9 36 1 35 12913.34000 12913.39288 -.052882 10 34 1 35 13011.80000 13011.74831 .051693 11 36 1 35 13154.87000 13155.06698 -.196982 12 34 1 35 13251.99000 13252.05480 -.064799 12 36 1 35 13274.58000 13274.61221 -.032210 11 35 1 36 13125.28000 13125.50221 -.222212 11 37 1 36 13148.75000 13148.85887 -.108871 12 35 1 36 13245.15000 13245.13929 .010705 12 37 1 36 13268.30000 13268.30987 -.009869 13 35 1 36 13364.05000 13363.96167 .088327 13 37 1 36 13386.94000 13386.95210 -.012102 14 35 1 36 13481.96000 13481.99850 -.038502 14 37 1 36 13504.80000 13504.81422 -.014221 15 35 1 36 13599.26000 13599.27296 -.012963 11 41 1 42 13080.83000 13080.87484 -.044843 11 43 1 42 13107.83000 13107.89770 -.067703 12 41 1 42 13199.98000 13199.92548 .054518 12 43 1 42 13226.78000 13226.73431 .045686 13 41 1 42 13318.11000 13318.18021 -.070207 14 41 1 42 13435.64000 13435.66658 -.026581 14 43 1 42 13462.06000 13462.06752 -.007515 15 41 1 42 13552.48000 13552.40619 .073812 15 43 1 42 13578.70000 13578.61208 .087921 9 44 1 45 12816.29000 12816.27131 .018691 9 46 1 45 12845.53000 12845.57820 -.048196 10 46 1 45 12965.52000 12965.73724 -.217237 10 46 1 45 12965.52000 12965.73724 -.217237 11 46 1 45 13085.01000 13085.04638 -.036376 11 46 1 45 13084.99000 13085.04638 -.056376 12 44 1 45 13175.02000 13174.94552 .074482 12 46 1 45 13203.60000 13203.54501 .054989 12 44 1 45 13175.03000 13174.94552 .084482 12 46 1 45 13203.64000 13203.54501 .094989 13 46 1 45 13321.08000 13321.26563 -.185630 13 46 1 45 13321.12000 13321.26563 -.145630 12 46 1 47 13157.43000 13157.42135 .008655 13 46 1 47 13274.98000 13275.14196 -.161964 14 46 1 47 13392.17000 13392.11061 .059390 14 48 1 47 13421.47000 13421.44213 .027870 15 46 1 47 13508.48000 13508.34735 .132652 13 58 1 59 13154.15000 13154.09594 .054063 13 60 1 59 13190.52000 13190.47814 .041858 14 60 1 59 13305.68000 13305.73182 -.051818 15 58 1 59 13384.40000 13384.44903 -.049033 15 60 1 59 13420.30000 13420.30418 -.004177 16 58 1 59 13498.56000 13498.60176 -.041756 16 60 1 59 13534.27000 13534.20461 .065394 13 67 1 66 13112.55000 13112.35694 .193060 14 65 1 66 13186.77000 13186.73793 .032072 14 67 1 66 13226.72000 13226.62005 .099947 15 65 1 66 13300.71000 13300.63232 .077676 15 67 1 66 13340.37000 13340.23211 .137890 16 65 1 66 13413.77000 13413.87389 -.103892 16 67 1 66 13453.21000 13453.19940 .010596 17 65 1 66 13526.37000 13526.46480 -.094796 17 67 1 66 13565.42000 13565.52318 -.103183 18 65 1 66 13638.31000 13638.40262 -.092619 18 67 1 66 13677.05000 13677.20011 -.150110 13 14 2 15 13266.08000 13266.12637 -.046367 13 16 2 15 13275.99000 13276.03055 -.040546 14 14 2 15 13385.40000 13385.44030 -.040296 14 16 2 15 13395.20000 13395.26806 -.068059 15 14 2 15 13503.97000 13503.95639 .013606 15 16 2 15 13513.65000 13513.70984 -.059836 16 14 2 15 13621.60000 13621.69595 -.095951 16 16 2 15 13631.27000 13631.37695 -.106952 17 14 2 15 13738.63000 13738.67521 -.045211 17 16 2 15 13748.25000 13748.28544 -.035437 18 14 2 15 13854.96000 13854.90584 .054164 18 16 2 15 13864.60000 13864.44674 .153262 19 14 2 15 13970.27000 13970.39537 -.125374 19 16 2 15 13979.77000 13979.86819 -.098191 20 14 2 15 14085.12000 14085.14772 -.027723 20 16 2 15 14094.46000 14094.55348 -.093479 21 14 2 15 14199.28000 14199.16360 .116402 21 16 2 15 14208.62000 14208.50310 .116897 22 14 2 15 14312.32000 14312.44100 -.120997 22 16 2 15 14321.65000 14321.71485 -.064848 23 14 2 15 14424.99000 14424.97566 .014335 23 16 2 15 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13496.70602 .173984 16 39 2 38 13520.46000 13520.37254 .087460 17 37 2 38 13612.35000 13612.34226 .007740 17 39 2 38 13635.84000 13635.83927 .000733 18 37 2 38 13727.30000 13727.25788 .042120 18 39 2 38 13750.63000 13750.58898 .041024 19 37 2 38 13841.49000 13841.45630 .033704 19 39 2 38 13864.63000 13864.62456 .005442 20 37 2 38 13954.88000 13954.93728 -.057280 20 39 2 38 13977.91000 13977.94525 -.035250 21 37 2 38 14067.68000 14067.69742 -.017419 21 39 2 38 14090.57000 14090.54711 .022889 21 39 2 38 14090.50000 14090.54711 -.047111 22 37 2 38 14179.75000 14179.73058 .019415 22 39 2 38 14202.38000 14202.42348 -.043478 23 39 2 38 14313.51000 14313.56544 -.055439 24 37 2 38 14401.50000 14401.58068 -.080678 24 39 2 38 14423.88000 14423.96229 -.082294 25 37 2 38 14511.33000 14511.37595 -.045950 25 39 2 38 14533.59000 14533.60202 -.012023 26 37 2 38 14620.56000 14620.40187 .158134 26 39 2 38 14642.21000 14642.47175 -.261751 27 37 2 38 14728.58000 14728.64569 -.065693 27 39 2 38 14750.47000 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-.013384 14 33 3 32 13122.55000 13122.45236 .097641 16 31 3 32 13336.56000 13336.48642 .073579 16 33 3 32 13356.53000 13356.57463 -.044633 17 31 3 32 13452.57000 13452.58224 -.012241 17 33 3 32 13472.58000 13472.52554 .054464 18 31 3 32 13567.97000 13567.94774 .022260 18 33 3 32 13587.77000 13587.74916 .020838 18 31 3 32 13567.93000 13567.94774 -.017740 18 33 3 32 13587.75000 13587.74916 .000838 19 31 3 32 13682.62000 13682.58777 .032232 19 33 3 32 13702.26000 13702.24991 .010086 19 31 3 32 13682.61000 13682.58777 .022232 20 31 3 32 13796.62000 13796.50352 .116475 20 33 3 32 13816.06000 13816.02854 .031458 20 31 3 32 13796.60000 13796.50352 .096475 20 33 3 32 13816.08000 13816.02854 .051458 21 31 3 32 13909.67000 13909.69303 -.023027 21 33 3 32 13929.09000 13929.08261 .007386 21 31 3 32 13909.67000 13909.69303 -.023027 21 33 3 32 13929.03000 13929.08261 -.052614 22 31 3 32 14022.19000 14022.15157 .038426 22 33 3 32 14041.48000 14041.40698 .073019 23 31 3 32 14133.90000 14133.87221 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13881.81000 13881.77857 .031432 22 38 3 39 13970.33000 13970.31352 .016484 22 40 3 39 13993.60000 13993.57379 .026211 23 38 3 39 14081.41000 14081.53432 -.124315 23 38 3 39 14081.37000 14081.53432 -.164315 23 40 3 39 14104.56000 14104.63510 -.075098 24 38 3 39 14191.90000 14192.00980 -.109797 24 40 3 39 14214.74000 14214.95152 -.211517 25 38 3 39 14301.80000 14301.72821 .071790 26 40 3 39 14433.22000 14433.29965 -.079650 27 38 3 39 14518.75000 14518.84302 -.093018 27 40 3 39 14541.34000 14541.30467 .035327 28 38 3 39 14626.17000 14626.21350 -.043501 28 40 3 39 14648.68000 14648.51236 .167642 29 38 3 39 14732.90000 14732.77602 .123979 30 38 3 39 14838.50000 14838.51921 -.019211 30 40 3 39 14860.55000 14860.48503 .064966 31 38 3 39 14943.45000 14943.43318 .016823 31 40 3 39 14965.28000 14965.22768 .052324 34 38 3 39 15253.07000 15253.13269 -.062692 34 40 3 39 15274.32000 15274.38744 -.067438 24 40 3 41 14175.06000 14175.17612 -.116124 24 42 3 41 14199.17000 14199.23311 -.063109 25 40 3 41 14284.63000 14284.73536 -.105358 25 42 3 41 14308.65000 14308.62599 .024012 26 40 3 41 14393.46000 14393.52426 -.064257 26 42 3 41 14417.18000 14417.24784 -.067837 27 42 3 41 14525.03000 14525.08454 -.054542 28 40 3 41 14608.73000 14608.73696 -.006964 28 42 3 41 14632.06000 14632.12207 -.062068 29 42 3 41 14738.21000 14738.34692 -.136921 30 40 3 41 14820.72000 14820.70964 .010359 30 42 3 41 14843.72000 14843.74662 -.026616 31 40 3 41 14925.52000 14925.45228 .067717 31 42 3 41 14948.43000 14948.31014 .119860 32 40 3 41 15029.52000 15029.35381 .166186 32 42 3 41 15052.26000 15052.02842 .231577 34 40 3 41 15234.57000 15234.61204 -.042045 Discarded lines (note that some of them are double). 5 29 0 30 12631.080000 5 31 0 30 12650.330000 5 31 0 30 12654.250000 7 39 0 40 12816.200000 7 39 0 40 12818.300000 11 41 0 40 13328.440000 11 41 0 40 13328.620000 10 36 0 37 13205.220000 5 27 0 28 12640.470000 5 27 0 28 12643.760000 5 29 0 28 12660.940000 7 61 0 62 12615.920000 6 14 0 15 12820.170000 6 16 0 15 12831.070000 9 14 0 15 13192.140000 9 14 0 15 13196.070000 9 16 0 15 13205.270000 9 16 0 15 13207.940000 13 71 0 72 13194.870000 13 73 0 72 13238.250000 14 71 0 72 13308.500000 11 34 1 35 13131.970000 7 66 0 65 12623.400000 9 64 0 65 12820.000000 13 44 1 45 13292.500000 10 44 1 45 12936.230000 13 44 1 45 13292.550000 0 40 2 41 11506.850000 0 42 2 41 11533.740000 0 42 2 41 11536.930000 1 40 2 41 11633.420000 1 40 2 41 11639.570000 1 42 2 41 11666.970000 7 42 2 41 12427.660000 5 32 2 33 12201.020000 8 32 2 33 12574.110000 8 34 2 33 12597.370000 3 16 1 17 12220.090000 6 16 1 17 12605.350000 4 62 0 63 12239.650000 5 62 0 63 12362.340000 7 62 0 63 12604.130000 2 21 2 20 11887.230000 5 19 2 20 12262.370000 5 21 2 20 12276.440000 2 28 3 29 11632.500000 2 28 3 29 11634.730000 5 30 3 29 12037.020000 5 30 3 29 12041.340000 5 30 2 31 12209.240000 5 30 2 31 12213.520000 5 32 2 31 12233.430000 8 32 2 31 12606.570000 8 32 2 31 12610.220000 2 24 2 25 11853.830000 2 24 2 25 11855.370000 5 24 2 25 12241.590000 5 24 2 25 12242.310000 5 26 2 25 12260.100000 8 24 2 25 12618.640000 8 26 2 25 12635.470000 3 16 2 17 12013.800000 6 16 2 17 12399.010000 6 18 2 17 12411.020000 1 36 2 35 11699.790000 8 34 2 35 12563.030000 8 36 2 35 12586.390000 1 36 3 37 11458.770000 1 36 3 37 11461.870000 0 52 2 53 11421.490000 0 54 2 53 11458.770000 2 54 2 53 11717.510000 9 52 2 53 12542.950000 10 36 0 37 13205.210000 18 21 2 20 13848.820000 13 40 2 41 13121.980000 16 40 2 41 13473.490000 20 32 2 33 13991.750000 20 32 2 33 13992.720000 18 48 2 49 13631.460000 18 17 2 18 13842.690000 18 17 2 18 13844.370000 19 65 1 66 13749.300000 19 67 1 66 13787.870000 20 65 1 66 13859.900000 20 67 1 66 13898.120000 13 39 2 38 13169.870000 14 30 2 29 13340.710000 14 30 2 29 13341.610000 14 30 1 29 13545.900000 14 30 1 29 13546.860000 14 30 1 29 13545.930000 13 43 1 42 13342.940000 13 43 1 42 13345.690000 29 40 2 41 14915.620000 21 24 2 25 14153.860000 21 24 2 25 14156.870000 24 26 2 25 14505.090000 24 26 2 25 14507.870000 27 24 2 25 14818.790000 27 24 2 25 14821.190000 21 18 2 17 14202.720000 27 29 2 30 14789.110000 30 31 2 30 15127.780000 23 37 2 38 14290.660000 23 37 2 38 14293.880000 29 39 2 38 14964.670000 29 30 2 29 15027.860000 30 30 2 29 15134.800000 21 19 2 20 14179.830000 24 21 2 20 14528.960000 30 30 3 29 14932.170000 21 19 2 18 14196.800000 21 19 2 18 14199.450000 24 26 2 27 14478.580000 24 26 2 27 14481.380000 24 28 2 27 14495.510000 24 28 2 27 14496.460000 27 28 2 27 14823.140000 27 28 2 27 14825.610000 23 36 2 35 14331.940000 23 36 2 35 14335.580000 26 34 2 35 14644.820000 29 36 2 35 14985.470000 29 36 2 35 14987.950000 21 22 2 23 14165.530000 21 22 2 23 14159.030000 21 24 2 23 14178.480000 21 24 2 23 14181.440000 24 22 2 23 14501.240000 24 22 2 23 14502.930000 27 24 2 23 14845.750000 29 40 3 41 14714.670000 Table 5. Ab initio potential energy curve of the A$^1\Sigma^+$ state of KLi resulting from calculations of Ref. [23]. Zero of energy is at the bottom of the ground state potential. R [A] E [cm-1] 1.58753190E+00 3.80295061E+04 1.64044963E+00 3.70723772E+04 1.69336736E+00 3.60735482E+04 1.74628509E+00 3.50391642E+04 1.90503828E+00 3.17725038E+04 1.95795601E+00 3.06455016E+04 2.01087374E+00 2.95097204E+04 2.06379147E+00 2.83735002E+04 2.11670920E+00 2.72451812E+04 2.16962693E+00 2.61344201E+04 2.22254466E+00 2.50499959E+04 2.27546239E+00 2.39993709E+04 2.32838012E+00 2.29897876E+04 2.38129785E+00 2.20258550E+04 2.48713331E+00 2.02503052E+04 2.54005104E+00 1.94421996E+04 2.59296877E+00 1.86880848E+04 2.64588650E+00 1.79873023E+04 2.69880423E+00 1.73389743E+04 2.75172196E+00 1.67413448E+04 2.80463969E+00 1.61926583E+04 2.85755742E+00 1.56907198E+04 2.91047515E+00 1.52328957E+04 2.96339288E+00 1.48172108E+04 3.01631061E+00 1.44410312E+04 3.06922834E+00 1.41019429E+04 3.12214607E+00 1.37975316E+04 3.17506380E+00 1.35256026E+04 3.22798153E+00 1.32837415E+04 3.28089926E+00 1.30699732E+04 3.33381699E+00 1.28823224E+04 3.38673472E+00 1.27183749E+04 3.43965245E+00 1.25770332E+04 3.49257018E+00 1.24558832E+04 3.54548791E+00 1.23538275E+04 3.59840564E+00 1.22691103E+04 3.65132337E+00 1.22001953E+04 3.70424110E+00 1.21459850E+04 3.75715883E+00 1.21053822E+04 3.81007656E+00 1.20768505E+04 3.86299429E+00 1.20595120E+04 3.91591202E+00 1.20524888E+04 3.96882975E+00 1.20549031E+04 4.02174748E+00 1.20656573E+04 4.07466521E+00 1.20840932E+04 4.12758294E+00 1.21097717E+04 4.18050067E+00 1.21415955E+04 4.23341840E+00 1.21793452E+04 4.28633613E+00 1.22223622E+04 4.33925386E+00 1.22702077E+04 4.39217159E+00 1.23224426E+04 4.44508932E+00 1.23786281E+04 4.49800705E+00 1.24383252E+04 4.55092478E+00 1.25015339E+04 4.60384251E+00 1.25675958E+04 4.65676024E+00 1.26367303E+04 4.70967797E+00 1.27082790E+04 4.76259570E+00 1.27822420E+04 4.81551343E+00 1.28586192E+04 4.86843116E+00 1.29371911E+04 4.92134889E+00 1.30177383E+04 4.97426662E+00 1.31000413E+04 5.02718435E+00 1.31843195E+04 5.08010208E+00 1.32703536E+04 5.13301981E+00 1.33581434E+04 5.18593754E+00 1.34474696E+04 5.23885527E+00 1.35381126E+04 5.29177300E+00 1.36302920E+04 5.34469073E+00 1.37237881E+04 5.39760846E+00 1.38186012E+04 5.45052619E+00 1.39145116E+04 5.50344392E+00 1.40117389E+04 5.55636165E+00 1.41096245E+04 5.60927938E+00 1.42086076E+04 5.66219711E+00 1.43084686E+04 5.71511484E+00 1.44089879E+04 5.76803257E+00 1.45101657E+04 5.82095030E+00 1.46117825E+04 5.87386803E+00 1.47136187E+04 5.92678576E+00 1.48161134E+04 5.97970349E+00 1.49186080E+04 6.03262122E+00 1.50213222E+04 6.08553895E+00 1.51238168E+04 6.13845668E+00 1.52265309E+04 6.19137441E+00 1.53288061E+04 6.24429214E+00 1.54308618E+04 6.29720987E+00 1.55322591E+04 6.35012760E+00 1.56334369E+04 6.40304533E+00 1.57339563E+04 6.45596306E+00 1.58335978E+04 6.50888079E+00 1.59328003E+04 6.56179852E+00 1.60309055E+04 6.61471625E+00 1.61279132E+04 6.66763398E+00 1.62240431E+04 6.72055171E+00 1.63190757E+04 6.77346944E+00 1.64130108E+04 6.82638717E+00 1.65054096E+04 6.87930490E+00 1.65967111E+04 6.93222263E+00 1.66864762E+04 6.98514036E+00 1.67747050E+04 7.03805809E+00 1.68613975E+04 7.09097582E+00 1.69465536E+04 7.14389355E+00 1.70299540E+04 7.19681128E+00 1.71118180E+04 7.24972901E+00 1.71917068E+04 7.30264674E+00 1.72700592E+04 7.35556447E+00 1.73462169E+04 7.40848220E+00 1.74206188E+04 7.46139993E+00 1.74932649E+04 7.51431766E+00 1.75637163E+04 7.56723539E+00 1.76324118E+04 7.62015312E+00 1.76989127E+04 7.67307085E+00 1.77634382E+04 7.72598858E+00 1.78257690E+04 7.77890631E+00 1.78863440E+04 7.83182404E+00 1.79447242E+04 7.88474177E+00 1.80011292E+04 7.93765950E+00 1.80555589E+04 8.46683680E+00 1.84936303E+04 8.99601410E+00 1.87708267E+04 9.52519140E+00 1.89389443E+04 1.00543687E+01 1.90403416E+04 2.11670920E+01 1.92369909E+04 2.64588650E+01 1.92383077E+04 3.17506380E+01 1.92385272E+04 3.70424110E+01 1.92387467E+04 4.23341840E+01 1.92387467E+04 5.29177300E+01 1.92387467E+04